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- Author:
- Shi, Chen; Shen, Xiuyu; Zhu, Yanan; Li, Xiaoqiang; Pang, Zengyuan; Ge, Mingqiao
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18548-18554
- ISSN:
- 1944-8252
- Subject:
- cations; color; fabrics; fluorescence; lead; manganese; terbium; ytterbium; yttrium
- Abstract:
- ... Luminescent materials have become prevalent in data communication and information security because of their special optical characteristics. Conventional luminescent materials generally exhibit unicolor emission and fixed excitation mode, resulting in decreased efficiency of anticounterfeiting applications. The development of an iridescent chameleon-like material that can change its emission color ...
- DOI:
- 10.1021/acsami.9b04213
-
http://dx.doi.org/10.1021/acsami.9b04213
- Author:
- Hu, He; Masarapu, Hema; Gu, Yuning; Zhang, Yifan; Yu, Xin; Steinmetz, Nicole F.
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18213-18223
- ISSN:
- 1944-8252
- Subject:
- Physalis; Physalis mottle virus; coat proteins; fluorescence; fluorescent dyes; gadolinium; humans; image analysis; magnetic resonance imaging; models; nanomedicine; nanoparticles; neoplasms; peptides; therapeutics
- Abstract:
- ... One of the greatest challenges in nanomedicine is the low efficiency with which nanoparticles are delivered to lesions such as tumors in vivo. Here, we show that Physalis mottle virus (PhMV)-like nanoparticles can be developed as bimodal contrast agents to achieve long circulation, specific targeting capability, and efficient delivery to tumors in vivo. The self-assembling coat protein nanostructu ...
- DOI:
- 10.1021/acsami.9b03956
- PubMed:
- 31074602
- PubMed Central:
- PMC7060085
-
http://dx.doi.org/10.1021/acsami.9b03956
- Author:
- Han, Dian-Dian; Wang, Zhen-Yu; Pan, Gui-Ling; Gao, Xue-Ping
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18427-18435
- ISSN:
- 1944-8252
- Subject:
- anions; anodes; cathodes; coordination compounds; electrochemistry; energy; energy density; gels; lithium; lithium batteries
- Abstract:
- ... A lithium–sulfur (Li–S) battery is widely regarded as one of the most promising technologies for energy storage because of its high theoretical energy density and cost advantage. However, the shuttling of soluble polysulfides between the cathode and the anode and the consequent lithium anode degradation strongly limit the safety and electrochemical performance in the Li–S battery. Herein, a metal– ...
- DOI:
- 10.1021/acsami.9b03682
-
http://dx.doi.org/10.1021/acsami.9b03682
- Author:
- Zhang, Bowen; Li, Wanli; Nogi, Masaya; Chen, Chuantong; Yang, Yang; Sugahara, Tohru; Koga, Hirotaka; Suganuma, Katsuaki
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18540-18547
- ISSN:
- 1944-8252
- Subject:
- adhesion; alloys; copper; copper nanoparticles; electrodes; electronics; energy; heaters; humidity; light intensity; nanosilver; nanowires; silver; temperature; thermal stability
- Abstract:
- ... In this paper, transparent electrodes with dense Cu@Ag alloy nanowires embedded in the stretchable substrates are successfully fabricated by a high-intensity pulsed light (HIPL) technique within one step. The intense light energy not only induces rapid mutual dissolution between the Cu core and the Ag shell to form dense Cu@Ag alloy nanowires but also embeds the newly formed alloy nanowires into t ...
- DOI:
- 10.1021/acsami.9b04169
-
http://dx.doi.org/10.1021/acsami.9b04169
- Author:
- Li, Chenxi; Li, Xuesong; Du, Xuewei; Tong, Tiezheng; Cath, Tzahi Y.; Lee, Jongho
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18456-18465
- ISSN:
- 1944-8252
- Subject:
- Fourier transform infrared spectroscopy; air; artificial membranes; contact angle; desalination; distillation; droplets; emulsions; energy; ethanol; fluorescence microscopy; fouling; hexane; hydrophilicity; nanoparticles; oils; petroleum; polymers; quartz; sodium chloride; wastewater; zwitterions
- Abstract:
- ... In this study, we develop Janus membranes comprising a hydrophilic zwitterionic polymer layer and an omniphobic (all-liquid-repelling) porous substrate that simultaneously possess fouling and wetting resistances. An omniphobic membrane was first fabricated by attaching silica nanoparticles (SiNPs) to the fibers of a quartz fiber mat, creating multilevel re-entrant structures, followed by surface f ...
- DOI:
- 10.1021/acsami.9b04212
-
http://dx.doi.org/10.1021/acsami.9b04212
- Author:
- Aksoy, Canan; Kaner, Papatya; Asatekin, Ayse; Çulfaz-Emecen, P. Zeynep
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18711-18719
- ISSN:
- 1944-8252
- Subject:
- calcium chloride; cleaning; fouling; humic acids; hydrophilicity; hydrophobicity; ionic strength; microgels; models; temperature; ultrafiltration
- Abstract:
- ... In this study, we show that codeposition of temperature responsive microgels in the foulant cake layer and cleaning of the cake upon stimuli-induced size change of the microgels is an effective method of fouling removal. Humic acid in CaCl₂ solution was used as a model foulant and poly(n-isopropylacrylamide) (p(NIPAm)) and poly(n-isopropylacrylamide-co-sulfobetainemethacrylate) (p(NIPAm-co-SBMA)) ...
- DOI:
- 10.1021/acsami.9b03217
-
http://dx.doi.org/10.1021/acsami.9b03217
- Author:
- Lin, Yuqing; Wu, Hao-Chen; Yasui, Tomoki; Yoshioka, Tomohisa; Matsuyama, Hideto
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18782-18796
- ISSN:
- 1944-8252
- Subject:
- composite polymers; coordination compounds; nanomaterials; permeability; ultrafiltration; wastewater treatment
- Abstract:
- ... Mixed-matrix membranes (MMMs) have been drawing increasing attention due to the high permeability and high rejection capabilities for highly efficient wastewater treatment applications. Nonetheless, improving the water permeance while maintaining the high rejection capability is still an ongoing challenge for the practically state-of-the-art MMMs. Herein, a new class of poly(ether sulfone) (PES) b ...
- DOI:
- 10.1021/acsami.9b04961
-
http://dx.doi.org/10.1021/acsami.9b04961
- Author:
- Kim, Juhee; Kang, Mingyun; Cho, Jangwhan; Yu, Seong Hoon; Chung, Dae Sung
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18580-18589
- ISSN:
- 1944-8252
- Subject:
- electronics; oxidants; polymers; reducing agents; solubility; transistors
- Abstract:
- ... One of the remaining keys to the success of polymer electronics is the ability to systematically pattern/stack polymer semiconductors with high precision. This paper reports the precise patterning and stacking of various polymer semiconductors with the assistance of a molecular oxidizing agent and reducing agent for donor and acceptor semiconductors, respectively. Such doping-induced solubility co ...
- DOI:
- 10.1021/acsami.9b03153
-
http://dx.doi.org/10.1021/acsami.9b03153
- Author:
- Ma, Zhihua; Lü, Jianhong; Dong, Wenyue; Ding, Junqiao; Wang, Lixiang
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18730-18738
- ISSN:
- 1944-8252
- Subject:
- aromatic amines; diphenylamine; hydrogen; iridium; ligands; phosphorescence; polymers
- Abstract:
- ... Three classes of red phosphorescent polymers (PF-H-x, PF-DPO-x, and PF-DPA-x, where x denotes the mole content of Ir complex) have been designed and synthesized, where the C∧N ligand of the tethered dopant bis(2,4-diphenylquinolyl)iridium(acetylacetonate) is substituted by hydrogen (H), diphenylphosphine oxide (DPO), and diphenylamine (DPA), respectively. It is found that the electron-withdrawing ...
- DOI:
- 10.1021/acsami.9b03618
-
http://dx.doi.org/10.1021/acsami.9b03618
- Author:
- Muniraj, Vedi Kuyil Azhagan; Dwivedi, Pravin Kumari; Tamhane, Parikshit Shivaji; Szunerits, Sabine; Boukherroub, Rabah; Shelke, Manjusha Vilas
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18349-18360
- ISSN:
- 1944-8252
- Subject:
- active sites; capacitance; electrochemistry; electrodes; electrolytes; energy; energy density; forces; graphene; texture
- Abstract:
- ... An effective and straightforward route for tailoring the self-supporting, exfoliated flexible graphite substrate (E-FGS) using electrochemical anodization is proposed. E-FGS has essential features of highly exfoliated, few-layered, two-dimensional graphite sheets with the size of several tens of micrometers, interconnected along the axis of the substrate surface. The novel hierarchical porous stru ...
- DOI:
- 10.1021/acsami.9b01712
-
http://dx.doi.org/10.1021/acsami.9b01712
- Author:
- He, Li; Fei, Fan; Wang, Wenbo; Song, Xuan
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18849-18857
- ISSN:
- 1944-8252
- Subject:
- biomimetics; ceramics; cracking; deformation; feedstocks; geometry; gravity; heat exchangers; manufacturing; photochemical reactions; polymerization; risk; surface quality
- Abstract:
- ... Ceramic stereolithography (CSL) is an additive manufacturing method for creating ceramic three-dimensional (3D) objects via the layer-by-layer photopolymerization of a ceramic suspension. A key challenge in CSL is that support structures are required for building overhanging structures to prevent part damage or deformation caused by gravity or process-induced shears. Removing the support structure ...
- DOI:
- 10.1021/acsami.9b04205
-
http://dx.doi.org/10.1021/acsami.9b04205
- Author:
- Feng, Wei; Qin, Fanglu; Yu, Miaomiao; Gao, Feng; Dai, Mingjin; Hu, Yunxia; Wang, Lifeng; Hou, Juan; Li, Bin; Hu, PingAn
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18511-18516
- ISSN:
- 1944-8252
- Subject:
- annealing; electronic equipment; nanosheets
- Abstract:
- ... Multilayer InSe has emerged as a promising candidate for applications in novel electronic and optoelectronic devices due to its direct bandgap, high electron mobility, and excellent photoresponse with a broad response range. Here, we report synthesis of superlattice InSe nanosheets by simple thermal annealing for the first time. The mobility is increased to 299.1 cm² V–¹ s–¹ for superlattice InSe ...
- DOI:
- 10.1021/acsami.9b01747
-
http://dx.doi.org/10.1021/acsami.9b01747
- Author:
- Tao, Jingying; Zhang, Yijie; Wang, Shengping; Wang, Ge; Hu, Fei; Yan, Xiaojun; Hao, Lifeng; Zuo, Zhijun; Yang, Xiaowei
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18342-18348
- ISSN:
- 1944-8252
- Subject:
- active sites; ambient temperature; catalysts; electrochemistry; electrodes; electrolytes; hydrogen production; iron; nanofibers; nickel; oxygen; oxygen production; surface area
- Abstract:
- ... Developing facile approaches to synthesize highly active and stable oxygen and hydrogen evolution electrocatalysts under mild conditions is crucial in water-splitting technology. Herein, Ni-nanofiber-based three-dimensional (3D) network is prepared by a magnetic-field-assisted reduction reaction and then a fast surface modification within only 3 s at room temperature is developed to prepare Fe@Ni- ...
- DOI:
- 10.1021/acsami.9b01431
-
http://dx.doi.org/10.1021/acsami.9b01431
- Author:
- Chen, Qian; Luo, Yu; Du, Wenxian; Liu, Zhuang; Zhang, Shengjian; Yang, Jiahui; Yao, Heliang; Liu, Tianzhi; Ma, Ming; Chen, Hangrong
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18133-18144
- ISSN:
- 1944-8252
- Subject:
- biocompatibility; biomineralization; bovine serum albumin; hydroxyl radicals; kidneys; liver; magnetic resonance imaging; nanoparticles; neoplasms; pH; photothermotherapy; sulfides; toxicity
- Abstract:
- ... Chemodynamic therapy (CDT) is an emerging field, which utilizes intratumoral iron-mediated Fenton chemistry for cancer therapy. However, the slightly acidic tumor environment is improper for the classical Fenton reaction, which is generally energetic in a narrow pH range (e.g., pH = 3–4). Herein, a kind of ultrasmall bovine serum albumin (BSA)-modified chalcopyrite nanoparticles (BSA-CuFeS₂ NPs) w ...
- DOI:
- 10.1021/acsami.9b02905
-
http://dx.doi.org/10.1021/acsami.9b02905
- Author:
- Huang, Yuqian; Wu, Shaohang; Chen, Rui; Fang, Shaoying; Zhang, Shasha; Wang, Gang; Chen, Wei
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18415-18422
- ISSN:
- 1944-8252
- Subject:
- chlorobenzene; gloves; hydrophobicity; methylamine; solar cells
- Abstract:
- ... Antisolvent and additive strategies are significantly positive to improve the crystal quality, device performance, and long-term stability of perovskite solar cells (PSCs). In addition, the high-quality perovskite thin films could be prepared by the methylamine (MA) gas-induced defect-healing process. However, until now, the research on adding MA into the antisolvent, which may take the advantages ...
- DOI:
- 10.1021/acsami.9b03323
-
http://dx.doi.org/10.1021/acsami.9b03323
- Author:
- Xie, Dong; Zhang, Junshen; Pan, Guoxiang; Li, Honggao; Xie, Shilei; Wang, Shoushan; Fan, Hongbo; Cheng, Faliang; Xia, Xinhui
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18662-18670
- ISSN:
- 1944-8252
- Subject:
- anodes; batteries; carbon nanotubes; cathodes; dopamine; electrical conductivity; electrochemistry; energy; foams; nanorods; nickel; porosity; sodium; strength (mechanics); surface area
- Abstract:
- ... Boosting electrochemical sodium storage properties is achieved by utilizing functionalized N-doped carbon nanotube arrays (NCNAs) as anode materials. The NCNA anodes are first fabricated by self-polymerization of dopamine on cobalt hydroxide nanorod arrays as the template. The NCNAs with diameters of 100–120 nm are grown vertically to Ni foam, forming self-supported nanotube arrays. Such a structu ...
- DOI:
- 10.1021/acsami.9b05667
-
http://dx.doi.org/10.1021/acsami.9b05667
- Author:
- Chang, Chao; Tao, Peng; Xu, Jiale; Fu, Benwei; Song, Chengyi; Wu, Jianbo; Shang, Wen; Deng, Tao
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18466-18474
- ISSN:
- 1944-8252
- Subject:
- Escherichia coli; Geobacillus stearothermophilus; ambient pressure; bacteria; evaporation; generators (equipment); heat; heat exchangers; indicator species; lighting; steam; temperature
- Abstract:
- ... Superheated solar steam generation above 100 °C is critical for many important applications such as sterilization but is challenging to achieve under natural fluctuating low-flux solar illumination and often requires pressurization and the usage of expensive optical concentrators. Herein, we demonstrate generation of superheated steam under ambient pressure and low-flux solar illumination by integ ...
- DOI:
- 10.1021/acsami.9b04535
-
http://dx.doi.org/10.1021/acsami.9b04535
- Author:
- Hillman, Febrian; Jeong, Hae-Kwon
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18377-18385
- ISSN:
- 1944-8252
- Subject:
- Fourier transform infrared spectroscopy; aluminum oxide; chemical bonding; metals; porosity; propane; propylene; sorption isotherms; topology
- Abstract:
- ... Zeolitic imidazolate frameworks (ZIFs) have gained much interest due to their potentials in gas separations. A hybrid approach by mixing metals and/or linkers has been recently investigated to fine-tune the ZIF framework porosity and surface properties and potentially extending their separation applications for many important gas mixtures. In general, the hybrid approach requires mixing of isostru ...
- DOI:
- 10.1021/acsami.9b02114
-
http://dx.doi.org/10.1021/acsami.9b02114
- Author:
- Lamport, Zachary A.; Broadnax, Angela D.; Scharmann, Ben; Bradford, Robert W.; DelaCourt, Andrew; Meyer, Noah; Li, Hui; Geyer, Scott M.; Thonhauser, Timo; Welker, Mark E.; Jurchescu, Oana D.
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18564-18570
- ISSN:
- 1944-8252
- Subject:
- aromatic compounds; diodes; electrodes; imines; moieties; silane; silicon
- Abstract:
- ... One of the simplest molecular-scale electronic devices is the molecular rectifier. In spite of considerable efforts aimed at understanding structure–property relationships in these systems, devices with predictable and stable electronic properties are yet to be developed. Here, we demonstrate highly efficient current rectification in a new class of compounds that form self-assembled monolayers on ...
- DOI:
- 10.1021/acsami.9b02315
-
http://dx.doi.org/10.1021/acsami.9b02315
- Author:
- Wang, Jiachen; Yang, Sennan; Ding, Peitao; Cao, Xiangyu; Zhang, Yue; Cao, Shitai; Zhang, Kuikui; Kong, Shixiao; Zhou, Yunlei; Wang, Xiaoliang; Li, Dongchan; Kong, Desheng
- Source:
- ACS applied materials & interfaces 2019 v.11 no.20 pp. 18590-18598
- ISSN:
- 1944-8252
- Subject:
- durability; electronics; gloves; manufacturing; medical equipment; robots; wafers
- Abstract:
- ... Stretchable electronics has emerged as a new class of electronic technology to expand the applications of conventional electronics built on rigid wafers. Among various systems, liquid-state devices utilize electronically active liquids to achieve excellent stretchability and durability. The widespread adaption to such attractive form of device is hindered by the lack of robust fabrication approach ...
- DOI:
- 10.1021/acsami.9b04730
-
http://dx.doi.org/10.1021/acsami.9b04730