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- Van der Kamp, Marc W., et al. Show all 6 Authors
- The Journal of physical chemistry 2016 v.120 no.44 pp. 11449-11463
- light harvesting complex; models; photosynthesis; physical chemistry; terminology
- ... Anisotropy pump–probe experiments have provided insights into the character of excitons formed in photosynthetic complexes. Rapid decay in the observed anisotropy is cited as evidence of the strength of coupling of the excitonic degrees of freedom to their environment. Here we show that ensemble averaging over realistic model Hamiltonians leads to a rapid decay of anisotropy to a value close to th ...