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1. Room-Temperature Tandem Condensation-Hydrogenation Catalyzed by Porous C₃N₄ Nanosheet-Supported Pd Nanoparticles

Author:
Goh, Tian Wei,   et al.   ; Nie, Renfeng; Chen, Minda; Pei, Yuchen; Zhang, Biying; Qi, Long; Chen, Jingwen; Qi, Zhiyuan; Zhang, Zhiguo; Huang, Wenyu;     Show all 10 Authors
Source:
ACS sustainable chemistry & engineering 2018 v.7 no.3 pp. 3356-3363
ISSN:
2168-0485
Subject:
ambient temperature; carbon nitride; catalysts; catalytic activity; cyclohexanones; hydrogen; hydrogenation; nanoparticles; nanosheets; nitriles; palladium; surface area
Abstract:
... Tandem catalysis, often inspired by biological systems, offers many advantages in the synthesis of highly functionalized small molecules. NH₂-grafted porous C₃N₄ nanosheet with rich N species and surface area of 138 m²/g was fabricated via a NH₃-exfoliation method. After supporting Pd nanoparticles, the resulting bifunctional catalyst (Pd/C₃N₄–NH₂) could catalyze a one-step tandem condensation-hyd ...
DOI:
10.1021/acssuschemeng.8b05531